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- <title>UTas ePrints - The effects of hardpan layers on the water chemistry from the leaching of pyrrhotite-rich tailings material</title>
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- <meta content="Gilbert, S.E." name="eprints.creators_name" />
- <meta content="Cooke, D.R." name="eprints.creators_name" />
- <meta content="Hollings, P." name="eprints.creators_name" />
- <meta content="sgilbert@utas.edu.au" name="eprints.creators_id" />
- <meta content="D.Cooke@utas.edu.au" name="eprints.creators_id" />
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- <meta content="2007-10-07 21:58:59" name="eprints.datestamp" />
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- <meta content="The effects of hardpan layers on the water chemistry from the leaching of pyrrhotite-rich tailings material" name="eprints.title" />
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- <meta content="260100" name="eprints.subjects" />
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- <meta content="Hardpan, Mine tailings,Column
- leaching, Pyrrhotite oxidation, Tasmania,
- Australia" name="eprints.keywords" />
- <meta content="The original publication is available at www.springerlink.com
- " name="eprints.note" />
- <meta content="Column leaching experiments were used to determine the effects of an iron-rich hardpan layer, on the rate of tailings oxidation and the composition of leachate waters, from the Renison Bell tailings dams in western Tasmania, Australia. One-meter-long PVC columns, filled with tailings,
- cover material (Cassiterite Flotation Tailings) and hardpan samples from the tailings dams, were leached over a period of 14 weeks. Under dry cover conditions, when hardpan was present, the solute loads peaked at 21–49 days (Fe at 2,294 ppm and SO4 2- at 4,700 ppm), and stabilised at much lower
- concentrations after 9 weeks. In contrast, the solute
- loads steadily increased over time in the column where hardpan was absent (SO4 -2 from 1,800 to 3,100 ppm, and Fe from 407 to 1,692 ppm). Under saturated cover conditions, the solute concentrations in the leachate also increased with time (SO4 2- from 1,900 to 17,000 ppm, and Fe from
- 480 to 8,500 ppm). The presence of a hardpan layer
- between the reactive tailings and cover material has
- been found to improve leachate water chemistry and
- lessen the rate of sulphide oxidation." name="eprints.abstract" />
- <meta content="2003-09" name="eprints.date" />
- <meta content="published" name="eprints.date_type" />
- <meta content="Environmental Geology" name="eprints.publication" />
- <meta content="44" name="eprints.volume" />
- <meta content="6" name="eprints.number" />
- <meta content="687-697" name="eprints.pagerange" />
- <meta content="10.1007/s00254-003-0810-5" name="eprints.id_number" />
- <meta content="TRUE" name="eprints.refereed" />
- <meta content="0943-0105" name="eprints.issn" />
- <meta content="http://dx.doi.org/10.1007/s00254-003-0810-5" name="eprints.official_url" />
- <meta content="Ahonen L, Tuovinen OH (1994) Solid-phase alteration and iron
- transformation in column bioleaching of a complex sulphide
- ore. In: Alpers CN, Blowes DW (eds) The environmental geochemistry
- of sulphide oxidation. American Chemical Society,
- ACS Symposium Series 550, Ontario, pp 79–89
- Bain JG, Blowes DW, Robertson WD, Frind EO (2000) Modelling
- of sulphide oxidation with reactive transport at a mine drainage
- site. J Contam Hydrol 41:23–47
- Bahatti TM, Bigham JM, Carlson L, Tuovinen OH (1993) Mineral
- products of pyrrhotite oxidation by Thiobacillus ferrooxidans.
- Appl Environ Microbiol 59:1984–1990
- Barham RJ (1997) Schwertmannite: a unique mineral, contains a
- replaceable ligand, transforms to jarosites, hematites and/or
- basic iron sulphate. J Mater Res 12:2751–2758
- Bigham JM (1994) Mineralogy of ochre deposits formed by sulphide
- oxidation. In: Blowes DW, Jambor JL (eds) The environmental
- geochemistry of sulphide mine-wastes: short course handbook.
- Mineralogical Association of Canada, Ontario, pp 103–132
- Bigham JM, Schwertmann U, Traina SJ, Winland RL, Wolf M
- (1996) Schwertmannite and the chemical modelling of iron in
- acid sulphate waters. Geochim Cosmochim Acta 60:2111–2121
- Blowes DW, Reardon EJ, Jambor JL, Cherry JA (1991) The formation
- and potential importance of cemented layers in inactive
- sulphide mine tailings. Geochim Cosmochim Acta 55:965–978
- Bureau of Meteorology, www.bom.gov.au
- Chermak JA, Runnells DD (1995) Self-sealing hardpan barriers to
- minimise infiltration of water into sulphide-bearing overburden,
- ore and tailings piles. Tailings and Mine Waste ’96, pp 265–273
- Cravotta CA (1994) Secondary iron-sulphate minerals as sources
- of sulphate and acidity. In: Alpers CN, Blowes DW (eds) The
- environmental geochemistry of sulphide oxidation. American
- Chemical Society, ACS Symposium Series 550, Ontario, pp 345–
- 364
- Elberling B, Nicholson RV, Scharer JM (1994) A combined kinetic
- and diffusion model for pyrite oxidation in tailings: a change in
- controls with time. J Hydrol 157:47–60
- Elberling B, Nicholson RV (1996) Field determination of sulphide
- oxidation rates in mine tailings. Water Resour Res 32:1773–1784
- Frau F (2000) The formation-dissolution-precipitation cycle of
- melanterite at the abandoned pyrite mine of Genna Luas in
- Sardinia, Italy: environmental implications. Mineral Mag
- 64:995–1006
- Janzen MP, Nicholson RV, Scharer JM (2000) Pyrrhotite reaction
- kinetics: reaction rates for oxidation by oxygen, ferric iron, and
- for nonoxidative dissolution. Geochim Cosmochim Acta
- 64:1511–1522
- Johnson RH, Blowes DW, Robertson WD, Jambor JL (2000) The
- hydrogeochemistry of the Nickel Rim Mine tailings impoundment.
- J Contam Hydrol 41:49–80
- Kalinkin AM, Forsling W, Makarov DV, Makarov VN (2000)
- Surface oxidation of synthetic pyrrhotite during wetting-drying
- treatment. J Environ Eng Sci 17:329–335
- Keith DC, Runnells DD (1995) Experimental simulation of waste
- rock weathering under unsaturated and saturated conditions at
- Iron Mountain, California. Tailings and Mine Waste ‘96, pp
- 351–360
- Light TS (1972) Standard solution for redox potential measurements.
- Anal Chem 44:1038–1039
- Lin Z, Herbert RB (1997) Heavy metal retention in secondary
- precipitates from a mine rock dump and underlying soil,
- Dalarna, Sweden. Environ Geol 33:1–12
- McGregor RG, Blowes DW, Jambor JL, Robertson WD (1998) The
- solid-phase controls on the mobility of heavy metals at the
- Copper Cliff tailings area, Sudbury, Ontario, Canada. J Contam
- Hydrol 33:247–271
- McSweeney K, Madison FW (1988) Formation of a cemented
- subsurface horizon in sulphidic minewaste. J Environ Qual
- 17:256–262
- Nicholson RV, Gillham RW, Cherry JA, Reardon EJ (1989)
- Reduction of acid generation in mine tailings through the use of moisture-retaining cover layers as oxygen barriers. Can Geotech
- J 28:1-8
- Nicholson RV, Scharer JM (1994) Laboratory studies of pyrrhotite
- oxidation kinetics. In: Alpers CN, Blowes DW (eds) The environmental
- geochemistry of sulphide oxidation. American
- Chemical Society, ACS Symposium Series 550, Ontario, pp 15–30
- Rose S, Elliott WC (2000) The effects of pH regulation upon the
- release of sulphate from ferric precipitates formed in acid mine
- drainage. Appl Geochem 15:27–34
- Shum M, Lavkulich LM (1999) Use of colour to estimate oxidised
- Fe content in mine waste rock. Environ Geol 37:281–289
- Stromberg B, Banwart S (1999) Weathering kinetics of waste rock
- from the Aitik copper mine, Sweden: scale dependent rate factors
- and pH controls in large column experiments. J Contam
- Hydrol 39:59–89
- Wang Y, Reardon EJ (2001) A siderite/limestone reactor to remove
- arsenic and cadmium from waste-waters. Appl Geochem
- 16:1241–1249
- Villalobos M, Trotz MA, Leckie JO (2001) Surface complexation
- modelling of carbonate effects on the adsorption of Cr(VI),
- Pb(II), and U(VI) on goethite. Environ Sci Technol 35:3849–
- 3856" name="eprints.referencetext" />
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- <meta content="Column leaching experiments were used to determine the effects of an iron-rich hardpan layer, on the rate of tailings oxidation and the composition of leachate waters, from the Renison Bell tailings dams in western Tasmania, Australia. One-meter-long PVC columns, filled with tailings,
- cover material (Cassiterite Flotation Tailings) and hardpan samples from the tailings dams, were leached over a period of 14 weeks. Under dry cover conditions, when hardpan was present, the solute loads peaked at 21–49 days (Fe at 2,294 ppm and SO4 2- at 4,700 ppm), and stabilised at much lower
- concentrations after 9 weeks. In contrast, the solute
- loads steadily increased over time in the column where hardpan was absent (SO4 -2 from 1,800 to 3,100 ppm, and Fe from 407 to 1,692 ppm). Under saturated cover conditions, the solute concentrations in the leachate also increased with time (SO4 2- from 1,900 to 17,000 ppm, and Fe from
- 480 to 8,500 ppm). The presence of a hardpan layer
- between the reactive tailings and cover material has
- been found to improve leachate water chemistry and
- lessen the rate of sulphide oxidation." name="DC.description" />
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- <h1 class="ep_tm_pagetitle">The effects of hardpan layers on the water chemistry from the leaching of pyrrhotite-rich tailings material</h1>
- <p style="margin-bottom: 1em" class="not_ep_block"><span class="person_name">Gilbert, S.E.</span> and <span class="person_name">Cooke, D.R.</span> and <span class="person_name">Hollings, P.</span> (2003) <xhtml:em>The effects of hardpan layers on the water chemistry from the leaching of pyrrhotite-rich tailings material.</xhtml:em> Environmental Geology, 44 (6). pp. 687-697. ISSN 0943-0105</p><p style="margin-bottom: 1em" class="not_ep_block"></p><table style="margin-bottom: 1em" class="not_ep_block"><tr><td valign="top" style="text-align:center"><a href="http://eprints.utas.edu.au/2057/1/Gilbert.Cooke.Hollings.ENVIROGEO.2003.pdf"><img alt="[img]" src="http://eprints.utas.edu.au/style/images/fileicons/application_pdf.png" class="ep_doc_icon" border="0" /></a></td><td valign="top"><a href="http://eprints.utas.edu.au/2057/1/Gilbert.Cooke.Hollings.ENVIROGEO.2003.pdf"><span class="ep_document_citation">PDF</span></a> - Full text restricted - Requires a PDF viewer<br />444Kb</td><td><form method="get" accept-charset="utf-8" action="http://eprints.utas.edu.au/cgi/request_doc"><input accept-charset="utf-8" value="2596" name="docid" type="hidden" /><div class=""><input value="Request a copy" name="_action_null" class="ep_form_action_button" onclick="return EPJS_button_pushed( '_action_null' )" type="submit" /> </div></form></td></tr></table><p style="margin-bottom: 1em" class="not_ep_block">Official URL: <a href="http://dx.doi.org/10.1007/s00254-003-0810-5">http://dx.doi.org/10.1007/s00254-003-0810-5</a></p><div class="not_ep_block"><h2>Abstract</h2><p style="padding-bottom: 16px; text-align: left; margin: 1em auto 0em auto">Column leaching experiments were used to determine the effects of an iron-rich hardpan layer, on the rate of tailings oxidation and the composition of leachate waters, from the Renison Bell tailings dams in western Tasmania, Australia. One-meter-long PVC columns, filled with tailings,
- cover material (Cassiterite Flotation Tailings) and hardpan samples from the tailings dams, were leached over a period of 14 weeks. Under dry cover conditions, when hardpan was present, the solute loads peaked at 21–49 days (Fe at 2,294 ppm and SO4 2- at 4,700 ppm), and stabilised at much lower
- concentrations after 9 weeks. In contrast, the solute
- loads steadily increased over time in the column where hardpan was absent (SO4 -2 from 1,800 to 3,100 ppm, and Fe from 407 to 1,692 ppm). Under saturated cover conditions, the solute concentrations in the leachate also increased with time (SO4 2- from 1,900 to 17,000 ppm, and Fe from
- 480 to 8,500 ppm). The presence of a hardpan layer
- between the reactive tailings and cover material has
- been found to improve leachate water chemistry and
- lessen the rate of sulphide oxidation.</p></div><table style="margin-bottom: 1em" cellpadding="3" class="not_ep_block" border="0"><tr><th valign="top" class="ep_row">Item Type:</th><td valign="top" class="ep_row">Article</td></tr><tr><th valign="top" class="ep_row">Additional Information:</th><td valign="top" class="ep_row">The original publication is available at www.springerlink.com
- </td></tr><tr><th valign="top" class="ep_row">Keywords:</th><td valign="top" class="ep_row">Hardpan, Mine tailings,Column
- leaching, Pyrrhotite oxidation, Tasmania,
- Australia</td></tr><tr><th valign="top" class="ep_row">Subjects:</th><td valign="top" class="ep_row"><a href="http://eprints.utas.edu.au/view/subjects/260100.html">260000 Earth Sciences > 260100 Geology</a></td></tr><tr><th valign="top" class="ep_row">ID Code:</th><td valign="top" class="ep_row">2057</td></tr><tr><th valign="top" class="ep_row">Deposited By:</th><td valign="top" class="ep_row"><span class="ep_name_citation"><span class="person_name">Mrs Katrina Keep</span></span></td></tr><tr><th valign="top" class="ep_row">Deposited On:</th><td valign="top" class="ep_row">08 Oct 2007 08:58</td></tr><tr><th valign="top" class="ep_row">Last Modified:</th><td valign="top" class="ep_row">09 Jan 2008 02:30</td></tr><tr><th valign="top" class="ep_row">ePrint Statistics:</th><td valign="top" class="ep_row"><a target="ePrintStats" href="/es/index.php?action=show_detail_eprint;id=2057;">View statistics for this ePrint</a></td></tr></table><p align="right">Repository Staff Only: <a href="http://eprints.utas.edu.au/cgi/users/home?screen=EPrint::View&eprintid=2057">item control page</a></p>
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